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Title Approaching circular economy through waste-to-blue hydrogen: Systems modeling and multi-objective optimization
ID_Doc 5161
Authors Qian, QM; Ren, JZ; He, C; Azzaro-Pantel, C
Title Approaching circular economy through waste-to-blue hydrogen: Systems modeling and multi-objective optimization
Year 2024
Published
DOI 10.1016/j.cej.2024.154660
Abstract Hydrogen is gaining increasing recognition as a clean and versatile energy carrier. The conversion of waste materials into energy or chemical products plays a crucial role in the circular economy paradigm. This study provides a comprehensive analysis of the waste-to-blue hydrogen process. The process entails co-gasification of a mixture of waste materials such as plastics and biomass. The system incorporates a rigorous modeling of the carbon capture process using a blended MDEA/PZ solvent to produce blue hydrogen. A multi-objective optimization framework is introduced to simultaneously minimize the levelized cost of hydrogen and the cradle-togate lifecycle endpoint value. The minimum levelized cost of hydrogen determined through this analysis is $3.02/kg, which substantiates the economic feasibility of the system under consideration. The minimum life cycle endpoint value is 247.23 mPt per kilogram of H2, 49.38 % lower than the conventional steam methane reforming technique. The observations indicate that increasing the mass fraction of biomass in the feedstock, raising the gasifying temperature, and lowering the oxygen-to-feed ratio have a positive influence on both the final levelized cost of hydrogen and the life cycle endpoint value. The Pareto curve provides decision-makers with valuable insights into the trade-off between the two objectives.
Author Keywords Waste-to-hydrogen; Low-carbon hydrogen production; Life cycle optimization; Multi-objective optimization; Carbon dioxide capture; Gasification
Index Keywords Index Keywords
Document Type Other
Open Access Open Access
Source Science Citation Index Expanded (SCI-EXPANDED)
EID WOS:001297132500001
WoS Category Engineering, Environmental; Engineering, Chemical
Research Area Engineering
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