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Scientific Article details

Title Direct Dry Carbonation of Mining and Industrial Wastes in a Fluidized Bed for Offsetting Carbon Emissions
ID_Doc 8633
Authors Coppola, A; Scala, F; Azadi, M
Title Direct Dry Carbonation of Mining and Industrial Wastes in a Fluidized Bed for Offsetting Carbon Emissions
Year 2022
Published Processes, 10.0, 3
DOI 10.3390/pr10030582
Abstract The direct dry mineral carbonation of selected mining and industrial wastes, using carbon dioxide derived from combustion flue gas, was evaluated. Specifically, coal fly ash from two Australian brown coal-fired power plants, red mud from the refinement of bauxite into alumina, and diamond tailings were considered, due to their relevant residual alkali content. These materials were tested in a laboratory-scale fluidized bed reactor at different temperatures (300-450 degrees C), in a reactive environment that simulated the typical CO2 concentration in a combustion flue gas. The experimental results showed a low, but still appreciable, CO2 capture capacity for three of the tested materials, which appears to be more favorable in the lower temperature range and with relatively fast kinetics, indicating the practical relevance of the process. One of the fly ashes exhibited a different behavior; starting at 350 degrees C, the sorbent began to release CO2, rather than absorb it. This suggested that the sorbent was already extensively carbonated by weathering before the tests. This study provides some evidence for the possible viability of recycling mining waste and for the circular economy in offsetting carbon emissions in the mining industry.
Author Keywords CO2 capture; mineral carbonation; fly ash; red mud; diamond tailings; fluidized bed
Index Keywords Index Keywords
Document Type Other
Open Access Open Access
Source Science Citation Index Expanded (SCI-EXPANDED)
EID WOS:000774338700001
WoS Category Engineering, Chemical
Research Area Engineering
PDF https://www.mdpi.com/2227-9717/10/3/582/pdf?version=1647501464
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